Title: On the Projection-Based Convexification of Some Spectral Sets Abstract: Given a finite-dimensional real inner-product space E and a closed convex cone K in R^n, we call $\lambda: E\to K$ a spectral map if (E, R^n, $\lambda$) forms a generalized Fan-Theobald-von Neumann (FTvN) system, and call S a spectral set if $S := \lambda^{-1}(C)$ for some C in R^n. We provide projection-based characterizations of clconv(S) (i.e., the closed convex hull of S) under two settings, namely, when C has no invariance property and when C has certain invariance properties. In the former setting, our approach is based on characterizing the bi-polar set of S, which allows us to judiciously exploit the properties of $\lambda$ via convex dualities. In the latter setting, our results complement the existing characterization of clconv(S) in Jeong and Gowda (2023), and unify and extend the related results in Kim et al. (2022) established for certain special cases of $\lambda$ and C.